When is the best time to call your credit card company and ask for a Credit Limit Increase?

. So do I call and ask them AFTER i've paid off my bill (in full) to show them that I can pay it off? Or do I call them while I have a balance owing to show them that I am in need of a credit limit increase? What do you suggest?
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I would do it any time but how much do you need? I would try after you pay the bill.
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